Unironed clothes have not been ironed(= made flat and smooth using a piece of equipment called an iron, that has a handle and a flat base and is usually heated with electricity).
She was dressed casually in an unironed blouse and jeans.
His shirt was unironed and his jacket covered with dust.他的衬衫没有熨烫，夹克上沾满了灰尘。
Synonym: unpressed
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My dad never once wore jeans, or an unironed shirt.
She felt ashamed that the children's school uniforms were unironed and dirty.
There were piles of unironed clothing lying around.